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To get a goat to charge, you’ll have to stand in front of it. You’ll want to do this in front of a tree, coal ore, copper ore, emerald ore, iron ore, packed ice, or stone, as these are the only blocks that will get a goat to drop one of its horns. The goat will then charge at you. You’ll want to move out of the way so that it runs into the block behind you.
Again, this may take a few tries, and if you don’t move out of the goat’s way it will attack you instead, causing damage.
Source: https://www.distractify.com/p/how-to-get-a-goat-horn-in-minecraft
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